<oai_dc:dc xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:oai_dc="http://www.openarchives.org/OAI/2.0/oai_dc/" xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xsi:schemaLocation="http://www.openarchives.org/OAI/2.0/oai_dc/ http://www.openarchives.org/OAI/2.0/oai_dc.xsd">
  <dc:creator>Jiang Y</dc:creator>
  <dc:creator>Feurer T</dc:creator>
  <dc:creator>Carron R</dc:creator>
  <dc:creator>Sevilla GT</dc:creator>
  <dc:creator>Moser T</dc:creator>
  <dc:creator>Pisoni S</dc:creator>
  <dc:creator>Erni R</dc:creator>
  <dc:creator>Rossell MD</dc:creator>
  <dc:creator>Ochoa M</dc:creator>
  <dc:creator>Hertwig R</dc:creator>
  <dc:creator>Tiwari AN</dc:creator>
  <dc:creator>Fu F</dc:creator>
  <dc:date>2020</dc:date>
  <dc:description xmlns:ns0="xml" ns0:lang="en">Four-terminal (4-T) tandem solar cells (e.g., perovskite/CuInSe2 (CIS)) rely on three transparent conductive oxide electrodes with high mobility and low free carrier absorption in the near-infrared (NIR) region. In this work, a reproducible In2O3:H (IO:H) film deposition process is developed by independently controlling H2 and O2 gas flows during magnetron sputtering, yielding a high mobility value up to 129 cm2 V-1 s-1 in highly crystallized IO:H films annealed at 230 °C. Optimization of H2 and O2 partial pressures further decreases the crystallization temperature to 130 °C. By using a highly crystallized IO:H film as the front electrode in NIR-transparent perovskite solar cell (PSC), a 17.3% steady-state power conversion efficiency and an 82% average transmittance between 820 and 1300 nm are achieved. In combination with an 18.1% CIS solar cell, a 24.6% perovskite/CIS tandem device in 4-T configuration is demonstrated. Optical analysis suggests that an amorphous IO:H film (without postannealing) and a partially crystallized IO:H film (postannealed at 150 °C), when used as a rear electrode in a NIR-transparent PSC and a front electrode in a CIS solar cell, respectively, can outperform the widely used indium-doped zinc oxide (IZO) electrodes, leading to a 1.38 mA/cm2 short-circuit current (Jsc) gain in the bottom CIS cell of 4-T tandems.</dc:description>
  <dc:format>application/pdf</dc:format>
  <dc:identifier>https://sonar.ch/global/documents/139396</dc:identifier>
  <dc:language>eng</dc:language>
  <dc:relation>info:eu-repo/semantics/altIdentifier/doi/10.1021/acsnano.0c03265</dc:relation>
  <dc:relation>info:eu-repo/semantics/altIdentifier/pmid/32459466</dc:relation>
  <dc:rights>info:eu-repo/semantics/openAccess</dc:rights>
  <dc:source>ACS nano. - 2020</dc:source>
  <dc:subject xmlns:ns1="xml" ns1:lang="en">carrier mobility</dc:subject>
  <dc:subject xmlns:ns2="xml" ns2:lang="en">hydrogenated indium oxide</dc:subject>
  <dc:subject xmlns:ns3="xml" ns3:lang="en">optical analysis</dc:subject>
  <dc:subject xmlns:ns4="xml" ns4:lang="en">perovskite</dc:subject>
  <dc:subject xmlns:ns5="xml" ns5:lang="en">tandem solar cell</dc:subject>
  <dc:title xmlns:ns6="xml" ns6:lang="en">High-Mobility In2O3:H Electrodes for Four-Terminal Perovskite/CuInSe2 Tandem Solar Cells.</dc:title>
  <dc:type>http://purl.org/coar/resource_type/c_6501</dc:type>
</oai_dc:dc>
