Flow induced crystallisation of penetrable particles.

Scacchi A; Brader JM

doi:10.1088/1361-648X/aaaa10

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Journal article

Flow induced crystallisation of penetrable particles.

Scacchi A Department of Physics, University of Fribourg, CH-1700 Fribourg, Switzerland.
Brader JM

2018-02-15

Published in:

Journal of physics. Condensed matter : an Institute of Physics journal. - 2018

English For a system of Brownian particles interacting via a soft exponential potential we investigate the interaction between equilibrium crystallisation and spatially varying shear flow. For thermodynamic state points within the liquid part of the phase diagram, but close to the crystallisation phase boundary, we observe that imposing a Poiseuille flow can induce nonequilibrium crystalline ordering in regions of low shear gradient. The physical mechanism responsible for this phenomenon is shear-induced particle migration, which causes particles to drift preferentially towards the center of the flow channel, thus increasing the local density in the channel center. The method employed is classical dynamical density functional theory.

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