Journal article
Dopant-Free Hole-Transporting Materials for Stable and Efficient Perovskite Solar Cells.
- Paek S Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Qin P Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Lee Y Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Cho KT Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Gao P Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Grancini G Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Oveisi E Interdisciplinary Centre for Electron Microscopy, École Polytechnique Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
- Gratia P Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Rakstys K Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- Al-Muhtaseb SA Department of Chemical Engineering, Qatar University, P.O. Box 2713, Doha, Qatar.
- Ludwig C ENAC IIE GR-LUD, École Polytechnique Fédérale de Lausanne, CH-1015, Lausanne, Switzerland.
- Ko J Department of New Material Chemistry, Korea University, Jochiwon, Chungnam, 339-700, South Korea.
- Nazeeruddin MK Group for Molecular Engineering of Functional Materials, École Polytechnique Fédérale de Lausanne, CH-1951, Sion, Switzerland.
- 2017-07-18
Published in:
- Advanced materials (Deerfield Beach, Fla.). - 2017
English
Molecularly engineered novel dopant-free hole-transporting materials for perovskite solar cells (PSCs) combined with mixed-perovskite (FAPbI3 )0.85 (MAPbBr3 )0.15 (MA: CH3 NH3+ , FA: NH=CHNH3+ ) that exhibit an excellent power conversion efficiency of 18.9% under AM 1.5 conditions are investigated. The mobilities of FA-CN, and TPA-CN are determined to be 1.2 × 10-4 cm2 V-1 s-1 and 1.1 × 10-4 cm2 V-1 s-1 , respectively. Exceptional stability up to 500 h is measured with the PSC based on FA-CN. Additionally, it is found that the maximum power output collected after 1300 h remained 65% of its initial value. This opens up new avenue for efficient and stable PSCs exploring new materials as alternatives to Spiro-OMeTAD.
- Language
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- English
- Open access status
- closed
- Identifiers
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- DOI 10.1002/adma.201606555
- PMID 28714259
- Persistent URL
- https://sonar.ch/global/documents/214716
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