Higher-Order Topology in Bismuth.
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Schindler F
Department of Physics, University of Zurich, Winterthurerstrasse 190, 8057 Zurich, Switzerland.
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Wang Z
Department of Physics, Princeton University, Princeton, New Jersey 08544, USA.
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Vergniory MG
Donostia International Physics Center, P. Manuel de Lardizabal 4, 20018 Donostia-San Sebastian, Spain.
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Cook AM
Department of Physics, University of Zurich, Winterthurerstrasse 190, 8057 Zurich, Switzerland.
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Murani A
LPS, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.
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Sengupta S
CSNSM, Univ. Paris-Sud, IN2P3, UMR 8609, F-91405 Orsay Cedex, France.
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Kasumov AY
LPS, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.
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Deblock R
LPS, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.
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Jeon S
Joseph Henry Laboratories and Department of Physics, Princeton University, Princeton, New Jersey 08544, USA.
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Drozdov I
Condensed Matter Physics and Materials Science Department, Brookhaven National Laboratory, Upton, New York 11973, USA.
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Bouchiat H
LPS, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.
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Guéron S
LPS, Univ. Paris-Sud, CNRS, UMR 8502, F-91405 Orsay Cedex, France.
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Yazdani A
Joseph Henry Laboratories and Department of Physics, Princeton University, Princeton, New Jersey 08544, USA.
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Bernevig BA
Joseph Henry Laboratories and Department of Physics, Princeton University, Princeton, New Jersey 08544, USA.
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Neupert T
Department of Physics, University of Zurich, Winterthurerstrasse 190, 8057 Zurich, Switzerland.
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English
The mathematical field of topology has become a framework to describe the low-energy electronic structure of crystalline solids. A typical feature of a bulk insulating three-dimensional topological crystal are conducting two-dimensional surface states. This constitutes the topological bulk-boundary correspondence. Here, we establish that the electronic structure of bismuth, an element consistently described as bulk topologically trivial, is in fact topological and follows a generalized bulk-boundary correspondence of higher-order: not the surfaces of the crystal, but its hinges host topologically protected conducting modes. These hinge modes are protected against localization by time-reversal symmetry locally, and globally by the three-fold rotational symmetry and inversion symmetry of the bismuth crystal. We support our claim theoretically and experimentally. Our theoretical analysis is based on symmetry arguments, topological indices, first-principle calculations, and the recently introduced framework of topological quantum chemistry. We provide supporting evidence from two complementary experimental techniques. With scanning-tunneling spectroscopy, we probe the unique signatures of the rotational symmetry of the one-dimensional states located at step edges of the crystal surface. With Josephson interferometry, we demonstrate their universal topological contribution to the electronic transport. Our work establishes bismuth as a higher-order topological insulator.
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Language
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Open access status
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green
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https://sonar.ch/global/documents/95322
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